Records contain meeting minutes and agendas for Leadership Council, CPSA, Board of Trustees, and the Library Department. Also contains correspondence, photographic materials, outreach materials, manuals, course information, and Baker Demonstration School materials.

Books on the kindergarten, education reform, and educational techniques dating from the mid-19th century. Some authors include Friedrich Froebel, Susan Blow and Kate Wiggins. See the NLU book catalog for individual titles and descriptions.

Geared towards alumnae and faculty, The National Magazine contains news and educational articles. Formerly known as the Alumnae News, Kindergarten Journal, News-Bulletin, Our Guidon, and NCE News, the publication became The National Magazine in 1973.